As rightly signalled K.R. Murthy the integral cannot be separated as such.
We shall take the limit for the lower index going to zero as
$$
\eqalign{
& \int_0^1 {f(x)dx} = \mathop {\lim }\limits_{a\; \to \;0^{\, + } }
\int_a^1 {\left( {\left\lfloor {{1 \over {3x}}} \right\rfloor
- {1 \over 3}\left\lfloor {{1 \over x}} \right\rfloor } \right)dx} = \cr
& = \mathop {\lim }\limits_{a\; \to \;0^{\, + } } \int_a^1 {\left\lfloor {{1 \over {3x}}} \right\rfloor dx}
- \mathop {\lim }\limits_{a\; \to \;0^{\, + } } {1 \over 3}\int_a^1 {\left\lfloor {{1 \over x}} \right\rfloor dx} = \cr
& = \mathop {\lim }\limits_{a\; \to \;0^{\, + } } {1 \over 3}\int_a^1 {\left\lfloor {{1 \over {3x}}} \right\rfloor d\left( {3x} \right)}
- \mathop {\lim }\limits_{a\; \to \;0^{\, + } } {1 \over 3}\int_a^1 {\left\lfloor {{1 \over x}} \right\rfloor dx} = \cr
& = {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } } \int_{3a}^3 {\left\lfloor {{1 \over y}} \right\rfloor d\left( y \right)}
- \mathop {\lim }\limits_{a\; \to \;0^{\, + } } {1 \over 3}\int_a^1 {\left\lfloor {{1 \over x}} \right\rfloor dx} = \cr
& = {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } }
\left( {\int_{3a}^\infty {\left\lfloor {{1 \over x}} \right\rfloor d\left( x \right)}
- \int_3^\infty {\left\lfloor {{1 \over x}} \right\rfloor d\left( x \right)}
- \int_a^\infty {\left\lfloor {{1 \over x}} \right\rfloor dx}
+ \int_1^\infty {\left\lfloor {{1 \over x}} \right\rfloor dx} } \right) = \cr
& = {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } } \left( {\int_1^3 {\left\lfloor {{1 \over x}} \right\rfloor dx}
- \int_a^{3a} {\left\lfloor {{1 \over x}} \right\rfloor dx} } \right) = \cr
& = - {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } } \int_a^{3a} {\left\lfloor {{1 \over x}} \right\rfloor dx} = \cr
& = - {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } } \int_a^{3a} {\left( {{1 \over x}
- \left\{ {{1 \over x}} \right\}} \right)dx} = \cr
& = - {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } } \left( {\ln {{3a} \over a}
- \int_a^{3a} {\left\{ {{1 \over x}} \right\}dx} } \right) = \cr
& = - {1 \over 3}\mathop {\lim }\limits_{a\; \to \;0^{\, + } } \left( {\ln {{3a} \over a}
- \int_a^{3a} {\left( {0 \le \left\{ {{1 \over x}} \right\} < 1} \right)dx} } \right) = \cr
& = - {1 \over 3}\ln 3 = {1 \over 3}\ln \left( {{1 \over 3}} \right) \cr}
$$