To make things a little bit easier, first factor $x$ (whose limit is $1$) out of the numerator, then use $x^4-1=(x-1)(x+1)(x^2+1)$ for the denominator:
\begin{align}
\lim_{x\to 1}\frac{\frac{4x^3-2x}{\sqrt{x^2-1}}\ln(x+\sqrt{x^2-1})-2x^2}{x^4-1}&=\lim_{x\to 1}\frac{\frac{4x^2-2}{\sqrt{x^2-1}}\ln(x+\sqrt{x^2-1})-2x}{x^4-1}\\
&=\frac{1}{4}\lim_{x\to 1}\frac{\frac{4x^2-2}{\sqrt{x^2-1}}\ln(x+\sqrt{x^2-1})-2x}{x-1}
\end{align}
Denote $t=x+\sqrt{x^2-1}$.
Using $\ln(1+x)=x-\frac{x^2}{2}+\frac{x^3}{3}+o(x^3)$ we can write
$$\ln(x+\sqrt{x^2-1})=\ln(1+(t-1))=(t-1)-\frac{(t-1)^2}{2}+\frac{(t-1)^3}{3}+o\left((t-1)^3\right).$$
Notice that $o\left((t-1)^3\right)=o\left((x-1)^{3/2}\right)$ so that substituting this back into the limit we get
$$\lim_{x\to 1}\frac{\frac{4x^2-2}{\sqrt{x^2-1}}\left(x+\sqrt{x^2-1}-1-\frac{(x+\sqrt{x^2-1}-1)^2}{2}+\frac{(x+\sqrt{x^2-1}-1)^3}{3}+o\left((x-1)^{3/2}\right)\right)-2x}{x-1}$$
where I put the factor $\frac{1}{4}$ aside for now. We have
$$\lim_{x\to 1} \frac{\frac{4x^2-2}{\sqrt{x^2-1}}o\left((x-1)^{3/2}\right)}{x-1}=0$$
and this is why we had to take $3$ terms from the Taylor series. So now we can consider just
$$\lim_{x\to 1}\frac{\frac{4x^2-2}{\sqrt{x^2-1}}\left(x+\sqrt{x^2-1}-1-\frac{(x+\sqrt{x^2-1}-1)^2}{2}+\frac{(x+\sqrt{x^2-1}-1)^3}{3}\right)-2x}{x-1}$$
which can be solved using standard techniques: simplifying we get
$$\frac{2}{3}\lim_{x\to 1} \frac{8x^4-10x^3-2x^2+5x-1+2\sqrt{x^2-1}(4x^3-5x^2+x+4)}{\sqrt{x^2-1}}$$
which is the same as
$$\frac{\sqrt{2}}{3}\lim_{x\to 1} \frac{8x^4-10x^3-2x^2+5x-1+2\sqrt{x^2-1}(4x^3-5x^2+x+4)}{\sqrt{x-1}}$$
putting $\frac{\sqrt{2}}{3}$ aside and using L'Hopital's rule we get
$$\lim_{x\to 1} 2\sqrt{x-1}\left(32x^3-30x^2-4x+5+2\sqrt{x^2-1}(12x^2-10x+1)\\
+\frac{2x(4x^3-5x^2+x+4)}{\sqrt{x^2-1}}\right)$$
everything drops and we are left just with
$$\lim_{x\to 1} \frac{4x\sqrt{x-1}(4x^3-5x^2+x+4)}{\sqrt{x^2-1}}=\lim_{x\to 1} \frac{4x(4x^3-5x^2+x+4)}{\sqrt{x+1}}=\frac{16}{\sqrt{2}}$$
Bringing back the constants we took out, the original limit equals $\frac{1}{4}\cdot\frac{\sqrt{2}}{3}\cdot\frac{16}{\sqrt{2}}=\frac{4}{3}$.