There is another question about expressing "at most one", but it extremely specific and doesn't seem applicable to other cases. For example, "for all smurfs, at most 2 of them are angry." How would you express such a statement in predicate logic? And also, how would you express "There is a day where more than one smurf is happy." Would it be something like:
Given $S$ is the set of all smurfs, and $D$ is the set of all days and Happy is the following predicate, $Happy(x):$ "$x$ is happy"
$\exists d \in D, \exists s_1, s_2 \in S, s_1 \neq s_2 \land Happy(s_1) \land Happy(s_2)$
Is the reason why this works because even if more than 2 smurfs were happy, the statement would still be true since there does indeed exist two that are happy?