I found this to be a very challenging problem, which is why I am providing an answer, even though the OP (i.e. original poster) hasn't really shown any work.
Further, the OP specifically indicated that Trigonometry is not to be used. The only way that I could solve the problem was to use Trigonometry.
It could well be that there is some elegant purely geometric construction that proves the problem. Anyway...
Tools
In the diagram below, which is not drawn to scale, the challenge is to show that $(y + z) = 120^\circ - 2a.$
$(y + z) = 180^\circ - 4a - 2b = (120^\circ - 2a) + (60^\circ - 2a - 2b).$
So, the problem has been reduced to showing that
$$(60^\circ - 2a - 2b) = 0 \iff a + b = 30^\circ \iff \sin(a + b) = \dfrac{1}{2}. \tag0 $$
Since $\triangle ABC$ is isosceles,
$$S = 2R\cos(2a+b). \tag1 $$
Let $T$ denote the length of line segment $\overline{CD}.$
Then,
$$S = R\cos(b) + T\cos(a + b). \tag2 $$
Using the Law of Sines, you have that
$$\frac{T}{\sin(b)} = \frac{R}{\sin(a + b)} \implies
T = \frac{R\sin(b)}{\sin(a + b)}. \tag3 $$
Combining (2) and (3) gives
$$S = R\cos(b) + \frac{R\cos(a+b)\sin(b)}{\sin(a + b)} \implies $$
$$ S = \frac{R\cos(b)\sin(a+b) + R\cos(a+b)\sin(b)}{\sin(a + b)}. \tag4$$
Using sum and difference formulas, (4) above simplifies to
$$ S = \frac{R\sin(a+2b)}{\sin(a + b)}. \tag5$$
Combining (1) and (5) gives:
$$\cos(2a + b) \times [2 \times \sin(a + b)] = \sin(a + 2b). \tag6 $$
So, the entire problem has been reduced to showing that (6) above implies the RHS of (0) above.
Let $\theta = (a + b) \implies $
- $(a + 2b) = (2\theta - a)$
- $(2a + b) = (\theta + a)$.
Also, using sum and difference formulas,
So, (6) above may be re-expressed as
$$\cos(\theta + a) \times 2 \times \sin(\theta) = \sin(2\theta - a). \tag7 $$
Using sum and difference formulas, the LHS of (7) above becomes
$$[\cos(\theta)\cos(a) - \sin(\theta)\sin(a)] \times 2\sin(\theta) $$
$$ = 2\sin(\theta)\cos(\theta)\cos(a) - 2\sin^2(\theta)\sin(a). \tag8 $$
Similarly, the RHS of (7) above becomes
$$\sin(2\theta)\cos(a) - \cos(2\theta)\sin(a) $$
$$ = 2\sin(\theta)\cos(\theta)\cos(a) - [1 - 2\sin^2(\theta)]\sin(a). \tag9 $$
Comparing (8) and (9) above, notice that the first term in each expression is identical. Therefore, as a direct implication of (7) above, you have that
$$ - 2\sin^2(\theta)\sin(a) = - [1 - 2\sin^2(\theta)]\sin(a) \implies $$
$$ 2\sin^2(\theta) = [1 - 2\sin^2(\theta)] \implies $$
$$ 4\sin^2(\theta) = 1 \implies \sin^2(\theta) = \dfrac{1}{4} \implies $$
$$\sin(\theta) = \dfrac{1}{2} \implies \sin(a + b) = \dfrac{1}{2}.$$
Therefore, the equation on the RHS of (0) above has been established.
